Effects of Composite Processing Methods on Wood Particle Development and Length Distribution: Consequences on Mechanical Properties of Wood-Thermoplastic Composites

Authors

  • Hassine Bouafif
  • Ahmed Koubaa
  • Patrick Perre
  • Alain Cloutier

Keywords:

Wood, fiber length, composites, compounding, injection molding, compression molding, extrusion

Abstract

The relationship between structure and properties of high-density polyethylene (HDPE) filled with wood particles and processing techniques—injection molding, compression molding, and extrusion—was investigated. Wood particles were hammer-milled, sieved, and compounded into pellets at 35% by weight with HDPE using a twin-screw extruder. Coupling agent (ethylene-maleic anhydride copolymer) was added at 2% by wood filler weight. The pellets were used to produce test samples using the three processing techniques. The sensitivity of jack pine and several other wood particles (eastern white cedar, black spruce, and jack pine bark) to composite processing was analyzed. Bark particles showed higher propensity to generate fines than wood particles, possibly because of a higher thermal sensitivity. The major reduction in mean particle length was found to occur in the compounding process. Extrusion and injection molding contributed to particle length reduction to a lesser extent. Conversely, compression molding did not cause significant damage to wood particles. Stiffness and strength increased linearly with weight-averaged length.

References

Ali R, Iannace S, Nicolais L (2003) Effect of processing conditions on mechanical and viscoelastic properties of biocomposites. J Appl Polym Sci 88(7):1637-1642.nASTM (2003a) D638-03, Standard test method for tensile properties of plastics. ASTM, West Conshohocken, PA.nASTM (2003b) D790-03, Standard test method for flexural properties of unreinforced and reinforced plastics and electrical insulating materials plastics. ASTM, West Conshohocken, PA.nASTM (2003c) D4703-03, Standard practice for compression molding thermoplastic materials into specimens, plaques, or sheets. ASTM, West Conshohocken, PA.nBalasuriya PW, Ye L, Mai YW (2001) Mechanical properties of wood flake-polyethylene composites. Part I: Effects of processing methods and matrix melt flow behaviour. Compos Part A-Appl S 32(5):619-629.nBarbosa SE, Kenny JM (2000) Processing of short-fiber reinforced polypropylene. I. Influence of processing conditions on the morphology of extruded filaments. Polym Eng Sci 40(1):11-22.nBigg DM (1985) Effect of compounding on the properties of short fiber reinforced injection moldable thermoplastic composites. Polym Polym Compos 6(1):20-28.nBledzki AK, Faruk O (2003) Wood fibre reinforced polypropylene composites: Effect of fibre geometry and coupling agent on physico-mechanical properties. Appl Compos Mater 10(6):365-379.nBledzki AK, Faruk O (2004) Wood fiber reinforced polypropylene composites: Compression and injection molding process. Polym-Plast Technol 43(3):871-888.nClemons CM, Caulfield DF, Giacomin AJ (1999) Dynamic fracture toughness of cellulose-fiber-reinforced polypropylene: Preliminary investigation of microstructural effects. J Elastom Plast 31(4):367-378.nFu SY, Hu X, Yue CY (1999) Effects of fiber length and orientation distributions on the mechanical properties of short-fiber-reinforced polymers—A review. Mater Sci Res Int 5(2):74-83.nFu SY, Lauke B (1996) Effects of fiber length and fiber orientation distributions on the tensile strength of short-fiber-reinforced polymers. Compos Sci Technol 56 (10):1179-1190.nFu SY, Yue CY, Hu X, Mai YW (2001) Characterization of fiber length distribution of short-fiber reinforced thermoplastics. J Mater Sci Lett 20(1):31-33.nGreen DW, Winandy JE, Kretschmann DE (1999) Mechanical properties of wood. In Wood handbook—Wood as an engineering material. Gen. Tech. Rep. FPL-GTR-113. USDA Forest Service, Forest Products Laboratory, Madison, WI. 463 pp.nGrillo J, Andersen P, Papazoglou E (1993) Experimental studies for optimizing screw and die design when compounding fiberglass strand on the co-rotating twin screw extruder. J Reinf Plast Comp 12(3):311-326.nHernandez JP, Raush T, Rios A, Strauss S, Osswald TA (2002) Analysis of fiber damage mechanisms during processing of reinforced polymer melts. Eng Anal Bound Elem 26(7):621-628.nJuhlin E, Chen X, Papathanasiou TD (2002) On the effects of fiber length and spatial distribution on the stiffness of short-fiber reinforced composites. Polym Polym Compos 10(3):205-210.nKasliwal SG, Jones JW (2004) Gentle compounding of natural fiber filled PVC composites. ANTEC 2004 Plastics: Annual Technical Conference, Vol 1:283-287.nKim YS, Guo G, Wang KH, Park CB, Maine FW (2004) Processing/structure/property relationships for artificial wood made from stretched PP/wood-fiber composites. ANTEC 2004 Plastics. Vol 2:1608-1613.nLee BJ, McDonald AG, James B (2001) Influence of fiber length on the mechanical properties of wood-fiber/polypropylene prepreg sheets. Mater Res Innov 4(2-3): 97-103.nLu JZ, Wu Q, Negulescu II (2005) Wood-fiber/high-densitypolyethylene composites: Coupling agent performance. J Appl Polym Sci 96(1):93-102.nNeagu RC, Gamstedt EK, Berthold F (2006) Stiffness contribution of various wood fibers to composite materials. J Composite Mater 40(8):663-699.nPark BD, Balatinecz JJ (1997) A comparison of compounding processes for wood-fiber/thermoplastic composites. Polym Polym Compos 18(3):425-431.nRobertson G, Olson J, Allen P, Chan B, Seth R (1999) Measurement of fiber length, coarseness, and shape with the fiber quality analyzer. TAPPI J 82(10):93-98.nStark NM, Matuana LM, Clemons CM (2004) Effect of processing method on surface and weathering characteristics of wood-flour/HDPE composites. J Appl Polym Sci 93(3):1021-1030.nSuzuki H (2003) Probabilistic study of visible length of fibers under the surface of a short fiber reinforced composite. Nippon Kikai Gakkai Ronbunshu. Trans Jpn Soc Mech Eng 69(4):719-726.nXanthos M (1983) Processing conditions and coupling agent effects in polypropylene/wood flour composites. Plast Rub Proc Appl 3(3):223-228.nYilmazer U, Cansever M (2002) Effects of processing conditions on the fiber length distribution and mechanical properties of glass fiber reinforced nylon-6. Polym Polym Compos 23(1):61-71.n

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2010-01-18

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